IndiumV3, Main, Repository, bibRecord, 001670

Polymer solar cells using chlorinated indium tin oxide electrodes with high work function as the anode

Identifieur interne : 001670 ( Main/Repository ); précédent : 001669; suivant : 001671

Polymer solar cells using chlorinated indium tin oxide electrodes with high work function as the anode

Auteurs : RBID : Pascal:12-0035522

Descripteurs français

Pascal (Inist)
- Cellule solaire organique, Electrode ITO, Travail sortie, Anode, Couche ITO, Addition étain, Polymère conducteur, Couche tampon, Couche active, Haute performance, Courant court circuit, Tension circuit ouvert, Facteur remplissage, Evaluation performance, Eclairement, Endommagement, Dégradation, Spectrométrie UV, Spectrométrie photoélectron, Alimentation ininterrompue, Spectre photoélectron RX, Chlore composé organique, Oxyde d'indium, Thiophène dérivé polymère, Acide butyrique, Ester, Composé du fullerène, Electronique puissance, Alimentation électrique, ITO.

English descriptors

KwdEn :
- Active layer, Anode, Buffer layer, Butyric acid, Conducting polymers, Damaging, Degradation, Ester, Fill factor, Fullerene compounds, High performance, ITO layers, Illumination, Indium oxide, Indium tin oxide electrode, Open circuit voltage, Organic chlorine compounds, Organic solar cells, Performance evaluation, Photoelectron spectrometry, Power electronics, Power supply, Short circuit currents, Thiophene derivative polymer, Tin addition, Ultraviolet spectrometry, Uninterruptible power supply, Work function, X-ray photoelectron spectra.

Abstract

This paper reports polymer solar cells (PSCs) using chlorinated indium tin oxide (Cl-ITO) substrates with high work function as the anode. There is no conducting polymer buffer layer between the Cl-ITO anode and the active layer in these PSCs. PSCs with P3HT:PCBM (P3HT=poly(3-hexylthiophene), PCBM=[6,6]-phenyl-C₆₁-butyric acid methyl ester) exhibited high photovoltaic performance, short-circuit current density (J_sc) of 9.91 mA/cm², open-circuit voltage (V_oc) of 0.57, fill factor (FF) of 0.69, and photovoltaic efficiency of 3.90% under AM1.5G illumination immediately after the device fabrication. The photovoltaic performance is comparable to that of normal PSCs with a conducting polymer buffer layer. But the photovoltaic efficiency of PSCs with Cl-ITO degrades quickly. The photovoltaic efficiency dropped to 3.43% and 3.24% just 10 and 20 min after the device fabrication, respectively. The reasons for the photovoltaic degradation were studied by ultraviolet photoelectron spectroscopy (UPS) and X-ray photoelectron spectroscopy (XPS). The work function of Cl-ITO decreases with time. The decrease in the work function of Cl-ITO is attributed to Cl desorption from the surface of ITO.

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Pascal:12-0035522

Le document en format XML

<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Polymer solar cells using chlorinated indium tin oxide electrodes with high work function as the anode</title>
<author><name>KUAN SUN</name>
<affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Department of Materials Science and Engineering, National University of Singapore</s1>
<s2>Singapore 117576</s2>
<s3>SGP</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>Singapour</country>
<orgName type="university">Université nationale de Singapour</orgName>
</affiliation>
</author>
<author><name sortKey="Ouyang, Jianyong" uniqKey="Ouyang J">Jianyong Ouyang</name>
<affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Department of Materials Science and Engineering, National University of Singapore</s1>
<s2>Singapore 117576</s2>
<s3>SGP</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
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<country>Singapour</country>
<orgName type="university">Université nationale de Singapour</orgName>
</affiliation>
</author>
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<publicationStmt><idno type="inist">12-0035522</idno>
<date when="2012">2012</date>
<idno type="stanalyst">PASCAL 12-0035522 INIST</idno>
<idno type="RBID">Pascal:12-0035522</idno>
<idno type="wicri:Area/Main/Corpus">002428</idno>
<idno type="wicri:Area/Main/Repository">001670</idno>
</publicationStmt>
<seriesStmt><idno type="ISSN">0927-0248</idno>
<title level="j" type="abbreviated">Sol. energy mater. sol. cells</title>
<title level="j" type="main">Solar energy materials and solar cells</title>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Active layer</term>
<term>Anode</term>
<term>Buffer layer</term>
<term>Butyric acid</term>
<term>Conducting polymers</term>
<term>Damaging</term>
<term>Degradation</term>
<term>Ester</term>
<term>Fill factor</term>
<term>Fullerene compounds</term>
<term>High performance</term>
<term>ITO layers</term>
<term>Illumination</term>
<term>Indium oxide</term>
<term>Indium tin oxide electrode</term>
<term>Open circuit voltage</term>
<term>Organic chlorine compounds</term>
<term>Organic solar cells</term>
<term>Performance evaluation</term>
<term>Photoelectron spectrometry</term>
<term>Power electronics</term>
<term>Power supply</term>
<term>Short circuit currents</term>
<term>Thiophene derivative polymer</term>
<term>Tin addition</term>
<term>Ultraviolet spectrometry</term>
<term>Uninterruptible power supply</term>
<term>Work function</term>
<term>X-ray photoelectron spectra</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Cellule solaire organique</term>
<term>Electrode ITO</term>
<term>Travail sortie</term>
<term>Anode</term>
<term>Couche ITO</term>
<term>Addition étain</term>
<term>Polymère conducteur</term>
<term>Couche tampon</term>
<term>Couche active</term>
<term>Haute performance</term>
<term>Courant court circuit</term>
<term>Tension circuit ouvert</term>
<term>Facteur remplissage</term>
<term>Evaluation performance</term>
<term>Eclairement</term>
<term>Endommagement</term>
<term>Dégradation</term>
<term>Spectrométrie UV</term>
<term>Spectrométrie photoélectron</term>
<term>Alimentation ininterrompue</term>
<term>Spectre photoélectron RX</term>
<term>Chlore composé organique</term>
<term>Oxyde d'indium</term>
<term>Thiophène dérivé polymère</term>
<term>Acide butyrique</term>
<term>Ester</term>
<term>Composé du fullerène</term>
<term>Electronique puissance</term>
<term>Alimentation électrique</term>
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<front><div type="abstract" xml:lang="en">This paper reports polymer solar cells (PSCs) using chlorinated indium tin oxide (Cl-ITO) substrates with high work function as the anode. There is no conducting polymer buffer layer between the Cl-ITO anode and the active layer in these PSCs. PSCs with P3HT:PCBM (P3HT=poly(3-hexylthiophene), PCBM=[6,6]-phenyl-C<sub>61</sub>
-butyric acid methyl ester) exhibited high photovoltaic performance, short-circuit current density (J<sub>sc</sub>
) of 9.91 mA/cm<sup>2</sup>
, open-circuit voltage (V<sub>oc</sub>
) of 0.57, fill factor (FF) of 0.69, and photovoltaic efficiency of 3.90% under AM1.5G illumination immediately after the device fabrication. The photovoltaic performance is comparable to that of normal PSCs with a conducting polymer buffer layer. But the photovoltaic efficiency of PSCs with Cl-ITO degrades quickly. The photovoltaic efficiency dropped to 3.43% and 3.24% just 10 and 20 min after the device fabrication, respectively. The reasons for the photovoltaic degradation were studied by ultraviolet photoelectron spectroscopy (UPS) and X-ray photoelectron spectroscopy (XPS). The work function of Cl-ITO decreases with time. The decrease in the work function of Cl-ITO is attributed to Cl desorption from the surface of ITO.</div>
</front>
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<fA11 i1="01" i2="1"><s1>KUAN SUN</s1>
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<fA11 i1="02" i2="1"><s1>OUYANG (Jianyong)</s1>
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<fA14 i1="01"><s1>Department of Materials Science and Engineering, National University of Singapore</s1>
<s2>Singapore 117576</s2>
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<sZ>2 aut.</sZ>
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<fC01 i1="01" l="ENG"><s0>This paper reports polymer solar cells (PSCs) using chlorinated indium tin oxide (Cl-ITO) substrates with high work function as the anode. There is no conducting polymer buffer layer between the Cl-ITO anode and the active layer in these PSCs. PSCs with P3HT:PCBM (P3HT=poly(3-hexylthiophene), PCBM=[6,6]-phenyl-C<sub>61</sub>
-butyric acid methyl ester) exhibited high photovoltaic performance, short-circuit current density (J<sub>sc</sub>
) of 9.91 mA/cm<sup>2</sup>
, open-circuit voltage (V<sub>oc</sub>
) of 0.57, fill factor (FF) of 0.69, and photovoltaic efficiency of 3.90% under AM1.5G illumination immediately after the device fabrication. The photovoltaic performance is comparable to that of normal PSCs with a conducting polymer buffer layer. But the photovoltaic efficiency of PSCs with Cl-ITO degrades quickly. The photovoltaic efficiency dropped to 3.43% and 3.24% just 10 and 20 min after the device fabrication, respectively. The reasons for the photovoltaic degradation were studied by ultraviolet photoelectron spectroscopy (UPS) and X-ray photoelectron spectroscopy (XPS). The work function of Cl-ITO decreases with time. The decrease in the work function of Cl-ITO is attributed to Cl desorption from the surface of ITO.</s0>
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Polymer solar cells using chlorinated indium tin oxide electrodes with high work function as the anode

Polymer solar cells using chlorinated indium tin oxide electrodes with high work function as the anode

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